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Metal cation removal by P(VC-r-AA) copolymer ultrafiltration membranes

Nachuan Wang, Jun Wang, Peng Zhang, Wenbin Wang, Chuangchao Sun, Ling Xiao, Chen Chen, Bin Zhao, Qingran Kong, Baoku Zhu

《化学科学与工程前沿（英文）》 2018年第12卷第2期页码 262-272 doi: 10.1007/s11705-017-1682-7

摘要： A series of amphiphilic copolymers containing poly(vinyl chloride-r-acrylic acid) (P(VC-r-AA) ) was synthesized and used to prepare membranes via a non-solvent induced phase separation method. The prepared membranes were characterized by scanning electron microscopy, X-ray photoelectron spectroscopy, and water contact angle and zeta potential measurements. The copolymer P(VC-r-AA) chains did not dissolved in a coagulation bath, indicating that the AA segments were completely retained within the membrane. Enriching degree of AA segments in surface layer was 2 for copolymer membrane. In addition, the introduction of AA segments made the membrane electronegative and hydrophilic so that the membrane was sensitive to the solution pH. The fouling resistance, adsorption of Cu(II), Cr(III) and Ce(IV) ions and the desorption properties of the membranes were also determined. The copolymer membranes exhibited good antifouling performance with a fouling reversibility of 92%. The membranes also had good adsorption capacities for Cu(II), Cr(III) and Ce(IV) ions. The optimal pH for Cu(II) adsorption was 6 and the copolymer membrane has potential applications for low concentration Cu(II) removal.

关键词： poly(vinyl chloride-r-acrylic acid) negatively charged PVC membrane anti-fouling heavy metal adsorption Cu(II) removal

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Effect of electrokinetic property of charged polyether sulfone membrane on bovine serum albumin fouling

Xiaorong Meng, Shanshan Huo, Lei Wang, Xudong Wang, Yongtao Lv, Weiting Tang, Rui Miao, Danxi Huang

《环境科学与工程前沿（英文）》 2017年第11卷第2期 doi: 10.1007/s11783-017-0907-9

摘要： Negatively charged CMPES and positively charged QAPES membranes were fabricated. Charge modification reduced the adhesion forces between PES UF membranes and BSA. QAPES-BSA / was weaker than that of CMPES-BSA at pH 3 and on the contrary at pH 9. Flux decline rate was positively correlated with the adhesion forces of membrane-BSA. Variation of adhesion was consistent with that of potential absolute values. Negatively charged carboxymethylated polyethersulfone (CMPES) and positively charged quaternized polyethersulfone (QAPES) ultrafiltration (UF) membranes were prepared by bulk chemical modification and non-solvent induced phase separation method. The effects of PES membrane interfacial electrokinetic property on the bovine serum albumin (BSA) membrane fouling behavior were studied with the aid of the membrane-modified colloidal atomic force microscopy (AFM) probe. Electrokinetic test results indicated that the streaming potential (D ) of QAPES membrane was not consistent with its expected value, however, within the pH range of 3–10, the potentials of two charged-modified PES membranes were more stable than the unmodified membrane. When pH value was 3, 4.7 or 9, the interaction behavior between charged PES membrane and BSA showed that there was significant linear correlation between the jump distance of membrane-BSA adhesion force ( ) and the potential absolute value. Charged modification significantly reduced the adhesion of PES membrane-BSA, and the adhesion data was good linear correlated with the flux decline rate in BSA filtration process, especially reflected in the CMPES membrane. The above experimental facts proved that the charged membrane interfacial electric double layer structure and its electrokinetic property had strong ties with the protein membrane fouling behavior.

关键词： Charged PES UF membrane BSA Electrokinetic characterization Adhesion force Jump distance

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Novel polyethyleneimine/TMC-based nanofiltration membrane prepared on a polydopamine coated substrate

Zhe Yang, Xiaoyu Huang, Jianqiang Wang, Chuyang Y. Tang

《化学科学与工程前沿（英文）》 2018年第12卷第2期页码 273-282 doi: 10.1007/s11705-017-1695-2

摘要： Most commercial NF membranes are negatively charged at the pH range of a typical feed solution. In order to enhance the removal of cations (such as Mg or Ca ), we utilized polyethyleneimine (PEI) and trimesoyl chloride (TMC) to perform interfacial polymerization reaction on a polydopamine coated hydrolyzed polyacrylonitrile substrate to obtain a positively charged nanofiltration membrane. Effects of polydopamine coating time, PEI concentration, TMC reaction time and concentration on the membrane physicochemical properties and separation performance were systematically investigated using scanning electron microscopy, streaming potential and water contact angle measurements. The optimal NF membrane showed high rejection for divalent ions (93.6±2.6% for MgSO , 92.4±1.3% for MgCl , and 90.4±2.1% for Na SO ), accompanied with NaCl rejection of 27.8±2.5% with a permeation flux of 17.2±2.8 L·m ·h at an applied pressure of 8 bar (salt concentrations were all 1000 mg·L ). The synthesized membranes showed promising potentials for the applications of water softening.

关键词： nanofiltration polyethyleneimine trimesoyl chloride polydopamine positively charged rejection layer

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用锥形量热仪研究细水雾抑制熄灭PVC火

黄鑫,刘江虹,张永丰,秦俊

《中国工程科学》 2006年第8卷第12期页码 102-106

摘要：

利用锥形量热仪和单流体细水雾系统研究了细水雾抑制PVC火的过程，并观察了重燃现象的发生，测量了实验中热释放速率及O₂，CO₂，CO和烟气的浓度变化，并对不同细水雾工作压力及不同热辐射流量下的结果进行了比较由实验可知细水雾能快速扑灭PVC火，且压力越大灭火越迅速，但是在灭火后停止施加细水雾会发生重燃现象，且重燃发生的时间长短与作用在燃料表面的水量有关。

关键词： PVC火细水雾热释放速率重燃

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Temporal evolution of charged and neutral nanoparticle concentrations during atmospheric new particle

E. Rohan Jayaratne, Buddhi Pushpawela, Lidia Morawska

《环境科学与工程前沿（英文）》 2016年第10卷第5期 doi: 10.1007/s11783-016-0862-x

摘要： Over 100 new particle formation events were studied. In 50 events, charged and neutral particles were not formed at the same time. In 42 of these events the charged particles formed before the neutral particles. Their subsequent growth rates were not determined by the particle charge. The result suggests that ion induced nucleation plays a role in particle formation. Time series of nanoparticle number concentration during new particle formation (NPF) events in the urban environment of Brisbane, Australia, showed that the formation of charged particles often occurred before that of neutral particles. We monitored 241 days during the calendar year 2012 over which NPF events were observed on 108 days. We studied the times at which the charged and neutral particle concentrations in the size range 1.8–3.2 nm reached their peak values and found that they were clearly different in 50 events with the peak neutral particle concentration lagging behind the charged particle concentration during 42 of these events with a mean time lag of 24±12 min. While the charged particles were more likely to form before the neutral particles, once formed, the growth rate of the particles did not depend on their charge. While ion-induced nucleation is not the dominant mechanism of NPF in the atmosphere, our observations suggest that the presence of ions in the atmosphere plays a role that cannot be ignored.

关键词： Charged particles Cluster ions Secondary particles Environmental pollution

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Shear wall layout optimization of tall buildings using Quantum Charged System Search

Siamak TALATAHARI, Mahdi RABIEI

《结构与土木工程前沿（英文）》 2020年第14卷第5期页码 1131-1151 doi: 10.1007/s11709-020-0660-1

摘要： This paper presents a developed meta-heuristic algorithm to optimize the shear walls of tall reinforced concrete buildings. These types of walls are considered as lateral resistant elements. In this paper, Quantum Charged System Search (QCSS) algorithm is presented as a new optimization method and used to improve the convergence capability of the original Charged System Search. The cost of tall building is taken as the objective function. Since the design of the lateral system plays a major role in the performance of the tall buildings, this paper proposes a unique computational technique that, unlike available works, focuses on structural efficiency or architectural design. This technique considers both structural and architectural requirements such as minimum structural costs, torsional effects, flexural and shear resistance, lateral deflection, openings and accessibility. The robustness of the new algorithm is demonstrated by comparing the outcomes of the QCSS with those of its standard algorithm.

关键词： Quantum Charged System Search shear wall layout optimization tall buildings

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APPLE SUMO E3 LIGASE MDSIZ1 NEGATIVELY REGULATES DROUGHT TOLERANCE

《农业科学与工程前沿（英文）》 2021年第8卷第2期

摘要：

Drought stress typically causes heavy losses in apple production and uncovering the mechanisms by which apple tolerates drought stress is important in apple breeding. MdSIZ1 is a SUMO (small ubiquitin-like modifier) E3 ligase that promotes SUMO binding to substrate proteins. Here, we demonstrate that MdSIZ1 in apple has a negative relationship with drought tolerance. MdSIZ1 RNAi transgenic apple trees had a higher survival rate after drought stress. During drought stress they had higher leaf water potential, reduced ion leakage, lower H₂O₂ and malondialdehyde contents, and higher catalase activity. In addition, MdSIZ1 RNAi transgenic plants had a higher net photosynthetic rate during the latter period of drought stress. Finally, the transgenic apple trees also altered expression levels of some microRNAs in response to drought stress. Taken together, these results indicate that apple MdSIZ1 negatively regulates drought stress by enhancing leaf water-holding capacity and antioxidant enzyme activity.

关键词： apple / drought tolerance / gene expression / MdSIZ1

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适用于田野调查的加勒比按实蝇信息素聚氯乙烯剂型 Article

Daniel Kuzmich, Zachary A. Kawagoe, Spencer S. Walse

《工程（英文）》 2021年第7卷第11期页码 1646-1650 doi: 10.1016/j.eng.2020.09.011

摘要：在本文中，我们研究了利用雄性加勒比按实蝇（Loew）信息素、(±)-anastrephin 和(±)-epianastrephin，形成聚氯乙烯（PVC）聚合物基质引诱剂进行陷阱部署的制备方法PVC聚合物圆盘（100 mg）分别含有10%（质量分数）的(±)-epianastrephin 和(±)-anastrephin，天然存在的非对映体比例为7∶3。

关键词：按实蝇按实蝇信息素 Epianastrephin PVC引诱剂控制释放

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APPLE SUMO E3 LIGASE MDSIZ1 NEGATIVELY REGULATES DROUGHT TOLERANCE

《农业科学与工程前沿（英文）》 2021年第8卷第4期页码 662-662 doi: 10.15302/J-FASE-2021408

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GDF15 negatively regulates chemosensitivity via TGFBR2-AKT pathway-dependent metabolism in esophageal

《医学前沿（英文）》 2023年第17卷第1期页码 119-131 doi: 10.1007/s11684-022-0949-7

摘要： Treating patients with esophageal squamous cell carcinoma (ESCC) is challenging due to the high chemoresistance. Growth differentiation factor 15 (GDF15) is crucial in the development of various types of tumors and negatively related to the prognosis of ESCC patients according to our previous research. In this study, the link between GDF15 and chemotherapy resistance in ESCC was further explored. The relationship between GDF15 and the chemotherapy response was investigated through in vitro and in vivo studies. ESCC patients with high levels of GDF15 expression showed an inferior chemotherapeutic response. GDF15 improved the tolerance of ESCC cell lines to low-dose cisplatin by regulating AKT phosphorylation via TGFBR2. Through an in vivo study, we further validated that the anti-GDF15 antibody improved the tumor inhibition effect of cisplatin. Metabolomics showed that GDF15 could alter cellular metabolism and enhance the expression of UGT1A. AKT and TGFBR2 inhibition resulted in the reversal of the GDF15-induced expression of UGT1A, indicating that TGFBR2-AKT pathway-dependent metabolic pathways were involved in the resistance of ESCC cells to cisplatin. The present investigation suggests that a high level of GDF15 expression leads to ESCC chemoresistance and that GDF15 can be targeted during chemotherapy, resulting in beneficial therapeutic outcomes.

关键词： GDF15 esophageal squamous cell carcinoma chemoresistance cellular metabolism TGFBR2 AKT

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Ductility loss of hydrogen-charged and releasing 304L steel

Yanfei WANG, Jianming GONG, Yong JIANG, Wenchun JIANG, Wang JIANG

《机械工程前沿（英文）》 2013年第8卷第3期页码 298-304 doi: 10.1007/s11465-013-0265-7

摘要：

The mechanical properties and fracture behavior of 304L austenitic stainless steel after cathodic hydrogen charging and hydrogen spontaneously releasing are investigated by tensile tests. Flat tensile specimens were cathodic hydrogen charged at various current densities. For each density, two specimens were charged at the same condition. When the charging process completed, one specimen was tensile immediately to fracture and the other was aged to release the hydrogen out of it and then was also tensile to fracture. The resulting tensile properties and micrographs of fracture surfaces of these specimens were evaluated and compared. The results show ductility loss occurred in the hydrogen-charged specimens and the loss increased as the current density increasing. After hydrogen releasing, the specimens recovered a certain extent but not all of its original ductility. Scanning electron microscope (SEM) micrographs of fracture surfaces reveal that irreversible damage had developed in the hydrogen-releasing specimens during the releasing process rather than the charging process. This consequence can be ascribed to the high tensile stress caused by non-uniform hydrogen distribution during hydrogen releasing.

关键词： hydrogen embrittlement ductility loss hydrogen releasing control strategy 304L austenitic stainless steel

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Combustion and emission characteristics of a turbo-charged common rail diesel engine fuelled with diesel-biodiesel-DEE

Ni ZHANG, Zuohua HUANG, Xiangang WANG, Bin ZHENG

《能源前沿（英文）》 2011年第5卷第1期页码 104-114 doi: 10.1007/s11708-011-0138-x

摘要： The combustion and emission characteristics of a turbo-charged, common rail diesel engine fuelled with diesel-biodiesel-DEE blends were investigated. The study reports that the brake-specific fuel consumption of diesel-biodiesel-DEE blends increases with increase of oxygenated fuel fractions in the blends. Brake thermal efficiency shows little variation when operating on different diesel-biodiesel-DEE blends. At a low load, the NO emission of the diesel-biodiesel-DEE blends exhibits little variation in comparison with the biodiesel fraction. The NO emission slightly increases with increase in the biodiesel fraction in diesel-biodiesel-DEE blends at medium load. However, the NO emission increases remarkably with increase of the biodiesel fraction at high load. Particle mass concentration decreases significantly with increase of the oxygenated-fuels fraction at all engine speeds and loads; particle number concentration decreases remarkably with increase of the oxygenated-fuels fraction. HC and CO emissions decrease with increasing oxygenated-fuels fraction in these blends.

关键词： Combustion particulate emissions diesel-biodiesel-DEE blend diesel engine

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APPLE SUMO E3 LIGASE MDSIZ1 NEGATIVELY REGULATES DROUGHT TOLERANCE

Baohua CHU, Jia SUN, Huan DANG, Ziqing MA, Shuang ZHAO, Qingmei GUAN, Xuewei LI

《农业科学与工程前沿（英文）》页码 247-261 doi: 10.15302/J-FASE-2021388

摘要： Drought stress typically causes heavy losses in apple production and uncovering the mechanisms by which apple tolerates drought stress is important in apple breeding. MdSIZ1 is a SUMO (small ubiquitin-like modifier) E3 ligase that promotes SUMO binding to substrate proteins. Here, we demonstrate that in apple has a negative relationship with drought tolerance. RNAi transgenic apple trees had a higher survival rate after drought stress. During drought stress they had higher leaf water potential, reduced ion leakage, lower H O and malondialdehyde contents, and higher catalase activity. In addition, RNAi transgenic plants had a higher net photosynthetic rate during the latter period of drought stress. Finally, the transgenic apple trees also altered expression levels of some microRNAs in response to drought stress. Taken together, these results indicate that apple MdSIZ1 negatively regulates drought stress by enhancing leaf water-holding capacity and antioxidant enzyme activity.

关键词： apple drought tolerance gene expression MdSIZ1

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用于可穿戴式人体助力和运动康复的人工肌肉 Review

Tian-yun DONG, Xiang-liang ZHANG, Tao LIU

《信息与电子工程前沿（英文）》 2018年第19卷第11期页码 1303-1315 doi: 10.1631/FITEE.1800618

摘要：介电弹性体（dielectric elastomers，DE）和聚氯乙烯（polyvinyl chloride，PVC）凝胶致动应变和致动应力大，响应速度快，驱动寿命长，在可穿戴式人体助力和运动康复领域具有很大应用潜力在这篇综述中，我们首先分别介绍DE和PVC凝胶的工作原理。接着，总结常用DE材料和PVC凝胶材料。然后，回顾这两种材料所需要的驱动电极和自传感系统。

关键词：人工肌肉；智能材料；介电弹性体（DE）；聚氯乙烯（PVC）凝胶；执行器；可穿戴式人体助力；运动康复

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Membrane fouling control by ultrasound in an anaerobic membrane bioreactor

SUI Pengzhe, WEN Xianghua, HUANG Xia

《环境科学与工程前沿（英文）》 2007年第1卷第3期页码 362-367 doi: 10.1007/s11783-007-0062-9

摘要： In this study, ultrasound was used to control the membrane fouling online in an anaerobic membrane bioreactor (AMBR). Short-term running experiments were carried out under different operating conditions to explore feasible ultrasonic parameters. The experimental results indicated that when the crossflow velocity was more than 1.0 m/s, membrane fouling could be controlled effectively only by hydrodynamic methods without ultrasound. When ultrasound was applied, an ultrasonic power range of 60–150 W was suitable for the membrane fouling control in the experimental system. The experimental results showed that the membrane fouling was controlled so well that membrane filtration resistance (Σ) could stay at 5 × 10 m for more than a week with the crossflow velocity of 0.75 m/s, which equaled the effect of crossflow velocity of more than 1.0 m/s without ultrasound.

关键词： membrane filtration filtration resistance different feasible ultrasonic anaerobic membrane